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Investigation of species transport in a gas diffusion layer of a polymer electrolyte membrane fuel cell through two-phase modelling.

Hossain, Mamdud; Islam, Sheikh Zahidul; Pollard, Patricia

Authors

Patricia Pollard



Abstract

A two-phase polymer electrolyte membrane fuel cell model has been developed to investigate transport of species in a gas diffusion layer taking into account effects of liquid water saturation. A set of governing equations for mass, momentum, species concentration involving oxygen, hydrogen, water vapour and liquid water together with electrochemical reaction equations have been solved under computational fluid dynamics technique. The effects of presence of liquid water on the effective diffusivity of species have been investigated. A thorough comparison study of liquid water saturation model using power law with various exponential factors and a percolation based model has been carried out. The simulation results show that the power law model with exponential factor of 2 provides a good representation of species diffusivity and produces much closer agreement with experimental cell voltage, while the percolation based model produces overprediction of cell voltage. The effects of isotropic and anisotropic permeability of gas diffusion layer have also been studied and the simulated results show that the high isotropic permeability or a combination of high in-plane and low through-plane permeability results in higher performance of a polymer electrolyte membrane fuel cell. The fuel cell performance significantly deteriorates with low in-plane and high through-plane permeability of gas diffusion layer.

Citation

HOSSAIN, M., ISLAM, S.Z., and POLLARD, P. 2013. Investigation of species transport in a gas diffusion layer of a polymer electrolyte membrane fuel cell through two-phase modelling. Renewable energy [online], 51, pages 404-418. Available from: https://doi.org/10.1016/j.renene.2012.10.008

Journal Article Type Article
Acceptance Date Oct 7, 2012
Online Publication Date Nov 6, 2012
Publication Date Mar 31, 2013
Deposit Date Jun 6, 2013
Publicly Available Date Jun 6, 2013
Journal Renewable energy
Print ISSN 0960-1481
Electronic ISSN 1879-0682
Publisher Elsevier
Peer Reviewed Peer Reviewed
Volume 51
Pages 404-418
DOI https://doi.org/10.1016/j.renene.2012.10.008
Keywords PEM fuel cell; Saturation; Diffusivity; Permeability; Anisotropy; Gas diffusion layer
Public URL http://hdl.handle.net/10059/823

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